by Coherent anti-Stokes Raman scattering (CARS) 13,14,15,16,17 is a third-order nonlinear optical process (a specific type of four-wave mixing (FWM) spectroscopy) that employs molecular coherence.. Abstract. In this review the basis, recent developments and applications of coherent anti-Stokes Raman scattering (CARS) in the fields of spectroscopy and microscopy are dialed with. The nonlinear susceptibility of the investigated molecule induced by pump and Stokes laser beams employed in the CARS technique is discussed.
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Coherent anti-Stokes Raman scattering (CARS) microscopy can provide high resolution, high speed, high sensitivity, and non-invasive imaging of specific biomolecules without labeling. In this review, we first introduce the principle of CARS microscopy, and then discuss its configuration, including that of the laser source and the multiplex CARS system. Finally, we introduce the applications of.. 1.. IntroductionCoherent anti-Stokes Raman scattering (CARS) spectroscopy has proven to be a valuable tool for measuring temperature and major-species concentration in gas-phase reacting flows [1], [2], [3], [4].However, implementation of this measurement technique in harsh chemical environments has been somewhat limited by the requirement to maintain spatial overlap between multiple laser.
